HU Wangjiang, CHEN Min, YANG Weifeng, ZHANG Run, QIU Yusheng, ZHENG Minfang. Low 210Pb in the upper thermocline in the Canadian Basin: scavenge process over the Chukchi Sea[J]. Acta Oceanologica Sinica, 2014, 33(6): 28-39. doi: 10.1007/s13131-014-0486-6
Citation: HU Wangjiang, CHEN Min, YANG Weifeng, ZHANG Run, QIU Yusheng, ZHENG Minfang. Low 210Pb in the upper thermocline in the Canadian Basin: scavenge process over the Chukchi Sea[J]. Acta Oceanologica Sinica, 2014, 33(6): 28-39. doi: 10.1007/s13131-014-0486-6

Low 210Pb in the upper thermocline in the Canadian Basin: scavenge process over the Chukchi Sea

doi: 10.1007/s13131-014-0486-6
  • Received Date: 2013-01-25
  • Rev Recd Date: 2013-04-13
  • 210Pb was measured during the 3rd Chinese National Arctic Research Expedition cruise to investigate its spatial pattern in the western Arctic Ocean, as well as its relation with the thermocline in the Canadian Basin. The specific activities varied from 0.04 to 2.72, <0.013 to 4.37, and 0.1 to 4.85 Bq/m3 for dissolved, particulate, and bulk 210Pb, respectively, corresponding to respective averages of 0.65, 0.43, and 1.08 Bq/m3. In the Canadian Basin, the minimum 210Pb activities occurred in the thermocline, which was characterized by low temperature of-1.52℃ and salinity of 33.1. Combining the spatial distribution of 210Pb and hydrographical characteristics in the western Arctic Ocean, this scenario was ascribed to the effective scavenging of 210Pb when the Pacific water flowed across the Chukchi Shelf. Quantitatively, this interpretation was supported by both the shorter residence times and higher scavenging efficiencies (SE) of dissolved 210Pb over the Chukchi Shelf. The highest SE values were observed in the Herald Shoal and bottom waters over the slope.
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  • Aagaard K, Coachman L, Carmack E. 1981. On the halocline of the Arctic Ocean. Deep-Sea Research Part A: Oceanographic Research Papers, 28(6): 529-545
    Bacon M P, Spencer D W, Brewer P G. 1976. 210Pb/226Ra and 210Po/210Pb disequilibria in seawater and suspended particulate matter. Earth and Planetary Science Letters, 32(2): 277-296
    Chen Min, Huang Yipu, Guo Laodong, et al. 2002. Biological productivity and carbon cycling in the Arctic Ocean. Chinese Science Bulletin, 47(12): 1037-1040
    Chen Min, Huang Yipu, Jin Mingming, et al. 2003. The isotope tracer in the formation mechanism of the upper and lower thermocline water in Canada Basin. Science in China (Series D), 33(2): 127-138
    Chen Min, Ma Qiang, Guo Laodong, et al. 2012. Importance of lateral transport processes to 210Pb budget in the eastern Chukchi Sea during summer 2003. Deep-Sea Research Part II: Topical Studies in Oceanography, 81-84: 53-62
    Chen Min, Xing Na, Huang Yipu, et al. 2008. The mean residence time of river water in the Canada Basin. Chinese Science Bulletin, 53(5): 777-783
    Chung Y. 1981. 210Pb and 226Ra distributions in the circumpolar waters. Earth and Planetary Science Letters, 55(2): 205-216
    Chung Y, Craig H. 1983. 210Pb in the Pacific: the GEOSECS measurements of particulate and dissolved concentrations. Earth and Planetary Science Letters, 65(2): 406-432
    Cochran J K. 1982. The oceanic chemistry of the U-and Th-series nuclides in the oceans. In: Ivanovich M, Harmon R S, eds. Uranium Series Disequilibrium: Applications to Environmental Problems. Oxford: Clarendon Press, 384-430
    Cochran J K, Hirschberg D J, Livingston H, et al. 1995. Natural and anthropogenic radionuclide distributions in the Nansen Basin, Arctic Ocean: scavenging rates and circulation timescales. Deep-Sea Research Part Ⅱ: Topical Studies in Oceanography, 42(6): 1495-1517
    Cochran J K, McKibbin-Vaughan T, Dornblaser M M, et al. 1990. 210Pb scavenging in the North Atlantic and North Pacific oceans. Earth and Planetary Science Letters, 97(3-4): 332-352
    Cornwell J C. 1985. Sediment accumulation rates in an Alaskan arctic lake using a modified 210Pb technique. Canadian Journal of Fisheries and Aquatic Sciences, 42(4): 809-814
    Dibb J E. 1992. The accumulation of 210Pb at Summit, Greenland since 1855. Tellus B, 44(1): 72-79
    Ekwurzel B, Schlosser P, Mortlock R A, et al. 2001. River runoff, sea ice meltwater, and Pacific water distribution and mean residence times in the Arctic Ocean. Journal of Geophysical Research, 106(C5): 9075-9092
    Fleer A P, Bacon M P. 1984. Determination of 210Pb and 210Po in seawater and marine particulate matter. Nuclear Instruments and Methods in Physics Research, 223(2-3): 243-249
    Glover D M, Reeburgh W S. 1987. Radon-222 and radium-226 in southeastern Bering Sea shelf waters and sediment. Continental Shelf Research, 7: 433-456
    He Wentao. 2012. Radium isotopes in the western Arctic Ocean and the Prydz Bay and its adjacent areas, Antarctic (in Chinese) [dissertation]. Xiamen: Xiamen University
    Hermanson M H. 1990. 210Pb and 137Cs chronology of sediments from small, shallow Arctic lakes. Geochimica et Cosmochimica Acta, 54(5): 1443-1451
    Huh C-A, Pisias N G, Kelley J M, et al. 1997. Natural radionuclides and plutonium in sediments from the western Arctic Ocean: sedimentation rates and pathways of radionuclides. Deep-Sea Research Part Ⅱ: Topical Studies in Oceanography, 44(8): 1725-1743
    Jin Mingming, Shi Jiuxin, Lu Yong, et al. 2005. Nutrient maximums related to low oxygen concentrations in the southern Canada Basin. Acta Oceanologica Sinica, 24(6): 88-96
    Jones E, Anderson L. 1986. On the origin of the chemical properties of the Arctic Ocean halocline. Journal of Geophysical Research, 91(C9): 10759-10767
    Kim G. 2001. Large deficiency of polonium in the oligotrophic ocean's interior. Earth and Planetary Science Letters, 192(1): 15-21
    Kinney P, Arhelger M E, Burrell D C. 1970. Chemical characteristics of water masses in the Amerasian Basin of the Arctic Ocean. Journal of Geophysical Research, 75(21): 4097-4104
    Kipphut G W. 1978. An investigation of sedimentary processes in lakes [dissertation]. New York: Columbia University
    Lepore K, Moran S, Smith J. 2009. 210Pb as a tracer of shelf-basin transport and sediment focusing in the Chukchi Sea. Deep-Sea Research Part II: Topical Studies in Oceanography, 56(17): 1305-1315
    Li Yanping. 2004. Radium geochemical behavior and its oceanic implication (in Chinese) [dissertation]. Xiamen: Xiamen University
    Ma Qiang, Chen Min, Qiu Yusheng, et al. 2005. Regional estimates of POC export flux derived from thorium-234 in the western Arctic Ocean. Acta Oceanologica Sinica, 24(6): 97-108
    Masqué P, Sanchez-Cabeza J, Bruach J, et al. 2002. Balance and residence times of 210Pb and 210Po in surface waters of the northwestern Mediterranean Sea. Continental Shelf Research, 22(15): 2127-2146
    McLaughlin F, Carmack E, Macdonald R, et al. 2004. The joint roles of Pacific and Atlantic-origin waters in the Canada Basin, 1997-1998. Deep-Sea Research Part Ⅰ: Oceanographic Research Papers, 51(1): 107-128
    Moore R M, Lowings M G, Tan F C. 1983. Geochemical profiles in the central Arctic Ocean: Their relation to freezing and shallow circulation. Journal of Geophysical Research, 88(C4): 2667-2674
    Moore R M, Smith J N. 1986. Disequilibria between 226Ra, 210Pb and 210Po in the Arctic Ocean and the implications for chemical modification of the Pacific water inflow. Earth and Planetary Science Letters, 77(3-4): 285-292
    Murray J W, Paul B, Dunne J P, et al. 2005. 234Th, 210Pb, 210Po and stable Pb in the central equatorial Pacific: Tracers for particle cycling. Deep-Sea Research Part Ⅰ: Oceanographic Research Papers, 52(11): 2109-2139
    Nozaki Y, Tsubota H, Kasemsupaya V, et al. 1991. Residence times of surface water and particle-reactive 210Pb and 210Po in the East China and Yellow seas. Geochimica et Cosmochimica Acta, 55: 1265-1272
    Nozaki Y, Tsunogai S. 1976. 226Ra, 210Pb and 210Po disequilibria in the western North Pacific. Earth and Planetary Science Letters, 32(2): 313-321
    Nozaki Y, Zhang Jing, Takeda A. 1997. 210Pb and 210Po in the equatorial Pacific and the Bering Sea: the effects of biological productivity and boundary scavenging. Deep-Sea Research Part Ⅱ: Topical Studies in Oceanography, 44(9-10): 2203-2220
    Roberts K A, Cochran J K, Barnes C. 1997. 210Pb and 239,240Pu in the Northeast Water Polynya, Greenland: particle dynamics and sediment mixing rates. Journal of Marine Systems, 10(1): 401-413
    Sarin M M, Kim G, Church T M. 1999. 210Po and 210Pb in the southequatorial Atlantic: distribution and disequilibrium in the upper 500 m. Deep-Sea Research Part Ⅱ: Topical Studies in Oceanography, 46(5): 907-917
    Shi Jiuxin, Zhao Jinping, Jiao Yutian, et al. 2004. Pacific inflow and its links with abnormal variations in the Arctic Ocean. Chinese Journal of Polar Research (in Chinese), 16(3): 253-260
    Shimada K, Itoh M, Nishino S, et al. 2005. Halocline structure in the Canada Basin of the Arctic Ocean. Geophysical Research Letters, 32(L03605): 1-5
    Smith J N, Moran S B, Macdonald R W. 2003. Shelf-basin interactions in the Arctic Ocean based on 210Pb and Ra isotope tracer distributions. Deep-Sea Research Part Ⅰ: Oceanographic Research Papers, 50(3): 397-416
    Thomson J, Turekian K K. 1976. 210Po and 210Pb distributions in ocean water profiles from the eastern South Pacific. Earth and Planetary Science Letters, 32(2): 297-303
    Weingartner T J, Aagaard K, Woodgate R A, et al. 2005. Circulation on the north central Chukchi Sea shelf. Deep-Sea Research Part Ⅱ: Topical Studies in Oceanography, 52(24-26): 3150-3174
    Weingartner T J, Cavalieri D J, Aagaard K, et al. 1998. Circulation, dense water formation, and outflow on the northeast Chukchi shelf. Journal of Geophysical Research, 103(C4): 7647-7661
    Weiss H, Naidu A. 1986. 210Pb flux in an arctic coastal region. Arctic, 39(1): 59-64
    Wilson C, Wallace D W R. 1990. Using the nutrient ratio NO/PO as a tracer of continental shelf waters in the central Arctic Ocean. Journal of Geophysical Research, 95(C12): 22193-22208
    Xing Na. 2002. Distribution of 226Ra, 228Ra and 210Pb in seawaters and their implication for marine geochemical processes (in Chinese) [dissertation]. Xiamen: Xiamen University
    Xing Na, Chen Min, Huang Yipu, et al. 2003. The distribution of 226Ra in the Arctic Ocean and the Bering Sea and its hydrologic implications. Science in China (Series D), 46(5): 516-528
    Yang Weifeng. 2005. Marine biogeochemistry of 210Po and 210Pb and their implications regarding the cycling and export of particles (in Chinese) [dissertation]. Xiamen: Xiamen University
    Yang Weifeng, Huang Yipu, Chen Min, et al. 2006. Disequilibria between 210Po and 210Pb in surface waters of the southern South China Sea and their implications. Science in China Series D: Earth Sciences, 49(1): 103-112
    Yang Weifeng, Huang Yipu, Chen Min, et al. 2009. Export and remineralization of POM in the Southern Ocean and the South China Sea estimated from 210Po/210Pb disequilibria. Chinese Science Bulletin, 54: 2118-2123
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