Source identification of aluminum in surface sediments of the Yellow Sea off the Shandong Peninsula

XU Gang; LIU Jian; PEI Shaofeng; KONG Xianghuai; HU Gang; GAO Maosheng

doi:10.1007/s13131-015-0766-9

山东半岛北部滨浅海区表层沉积物铝物源鉴别

doi: 10.1007/s13131-015-0766-9

1.
国土资源部青岛海洋地质研究所, 青岛 266071;海洋国家实验室海洋地质过程与环境功能实验室, 青岛 266061;国土资源部海洋油气资源与环境地质重点实验室, 青岛 266071;中国地质调查局滨海湿地生物地质重点实验室青岛 266071
2.
国土资源部青岛海洋地质研究所, 青岛 266071;中国地质调查局滨海湿地生物地质重点实验室青岛 266071

基金项目: The National Natural Science Foundation of China under contract Nos 41406078, 41330964, 41306175 and 41206073; the Science and Technology Development Fund Project in Shinan District of Qingdao, Shandong Province, China under contract No. 2013-14-007-JY; the China Geological Survey Bureau, the Ministry of Land and Natural Resources of China under contract No. GZH201200505.

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- 收稿日期: 2014-10-30
- 修回日期: 2015-03-02

Source identification of aluminum in surface sediments of the Yellow Sea off the Shandong Peninsula

1.
Qingdao Institute of Marine Geology, Ministry of Land and Natural, Qingdao 266071, China;Laboratory for Marine Geology, Qingdao National Laboratory for Marine Science and Technology, Qingdao 266061, China;Key Laboratory of Ministry of Land and Natural Resources for Marine Hydrocarbon Resources and Environment Geology, Qingdao 266071, China;Key Laboratory of China Geological Survey Bureau for Coastal Wetland Biogeosciences, Qingdao 266071, China
2.
Qingdao Institute of Marine Geology, Ministry of Land and Natural, Qingdao 266071, China;Key Laboratory of China Geological Survey Bureau for Coastal Wetland Biogeosciences, Qingdao 266071, China

摘要

摘要: 本文对采自山东半岛北部近岸海域的表层沉积物进行了粒度和元素测试分析。分析结果表明:研究区表层沉积物主要由粉砂粒级组分构成,其粒度特征同黄河相似。本区表层沉积物中元素铝含量变化范围介于5.57%~7.37%之间,平均含量为6.33±0.40%;此外,其平面变化特征主要受粒度控制。铝钛比值、铝含量、钛含量以及平均粒径之间的相关性分析表明本区表层沉积物中的铝主要来源于陆源碎屑物质的供应,同时还受部分人为源物质的影响。在研究区某些站位,铝钛比值由于受到人为源过剩铝的影响而远大于黄土物质背景值。因此,即使在以陆源碎屑沉积为主的近岸沉积物中运用铝元素作为陆源物质指标时,也应该首先对沉积物中的铝来源进行鉴别。
- 铝 /
- 物源鉴别 /
- 表层沉积物 /
- 山东半岛 /
- 黄海
Abstract: Surface sediment samples in the near shore area of the north Shandong Peninsula are collected for grain size and element analyses. The results indicate that the surface sediments in the study area are primarily composed of the silt-sized components similar to the Huanghe River. The total concentration of aluminum varies from 5.57% to 7.37% (average (6.33±0.40)%), and its spatial distribution is mainly controlled by the grain size. Correlations between the ratio of aluminum to titanium concentration and aluminum concentration, titanium concentration and the mean grain size indicate that aluminum in the near shore surface sediments is affected majorly by the terrigenous source, and partially by the anthropogenic source. The ratios of aluminum to titanium concentrations are larger than the background value of loess matter at some stations due to the existence of excess aluminum associated with human activities. Thus, the sources of aluminum should be identified firstly when aluminum is used as an index of terrigenous matter even in the near shore area dominated by terrigenous deposits.
- aluminum /
- source identification /
- surface sediments /
- Shandong Peninsula /
- Yellow Sea

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参考文献(37)

Arz H W, Pätzold J, Wefer G. 1998. Correlated millennial-scale changes in surface hydrography and terrigenous sediment yield inferred from last-glacial marine deposits off Northeastern Brazil. Quaternary Research, 50(2):157-166

Chen H F, Song Shengrong, Lee T Q, et al. 2010. A multiproxy lake record from Inner Mongolia displays a late Holocene teleconnec-tion between Central Asian and North Atlantic climates. Quaternary International, 227(2):170-182

Chen H F, Chang Yuanpin, Kao S J, et al. 2011. Mineralogical and geochemical investigations of sediment-source region changes in the Okinawa Trough during the past 100 ka (IMAGES core MD012404). Journal of Asian Earth Sciences, 40(6):1238-1249

Chen H F, Yeh P Y, Song Shengrong, et al. 2013. The Ti/Al molar ratio as a new proxy for tracing sediment transportation processes and its application in aeolian events and sea level change in East Asia. Journal of Asian Earth Sciences, 73:31-38

China National Environmental Monitoring Center (CNEMC). 1990.

Chinese Elemental Background Values for soils (in Chinese).Beijing:Chinese Environmental Science Press, 283-290

Din Z B. 1992. Use of aluminium to normalize heavy-metal data from estuarine and coastal sediments of Straits of Melaka. Marine Pollution Bulletin, 24(10):484-491

Dymond J, Suess E, Lyle M. 1992. Barium in deep-sea sediment:A geochemical proxy for paleoproductivity. Paleoceanography, 7(2):163-181

Dymond J, Collier R, McManus J, et al. 1997. Can the aluminum and titanium contents of ocean sediments be used to determine the paleoproductivity of the oceans?. Paleoceanography, 12(4):586-593

Folk R L, Ward W C. 1957. Brazos river bar:a study in the significance of grain size parameters. Journal of Sedimentary Research, 27(1):3-26

Hu D X, Li Y X. 1993. Study of ocean circulation. In:Tseng C K, Zhou H O, Li B C, eds. Marine Science Study and its Prospect in China. Qingdao:Qingdao Publishing House, 513-516

Jansen J H F, Van der Gaast S J, Koster B, et al. 1998. CORTEX, a shipboard XRF-scanner for element analyses in split sediment cores. Marine Geology, 151(1-4):143-153

Klump J, Hebbeln D, Wefer G. 2000. The impact of sediment provenance on barium-based productivity estimates. Marine Geology, 169(3-4):259-271

Liu Jian, Saito Y, Wang Hong, et al. 2007. Sedimentary evolution of the Holocene subaqueous clinoform off the Shandong Peninsula in the Yellow Sea. Marine Geology, 236(3-4):165-187

Liu Jian, Saito Y, Kong Xianghuai, et al. 2009. Geochemical characteristics of sediment as indicators of post-glacial environmental changes off the Shandong Peninsula in the Yellow Sea. Continental Shelf Research, 29(7):846-855

Liu J P, Milliman J D, Gao Shu. 2002. The Shandong mud wedge and post-glacial sediment accumulation in the Yellow Sea. Geo-Marine Letters, 21(4):212-218

Liu J P, Milliman J D, Gao Shu, et al. 2004. Holocene development of the Yellow River's subaqueous delta, North Yellow Sea. Marine Geology, 209(1-4):45-67

Murray R W, Leinen M, Isern A R. 1993. Biogenic flux of Al to sediment in the central equatorial Pacific Ocean:Evidence for increased productivity during glacial periods. Paleoceanography, 8(5):651-670

Murray R W, Leinen M. 1996. Scavenged excess aluminum and its relationship to bulk titanium in biogenic sediment from the central equatorial Pacific Ocean. Geochimica et Cosmochimica Acta, 60(20):3869-3878

Paerl H W. 1999. Cultural eutrophication of shallow coastal waters:coupling changing anthropogenic nutrient inputs to regional management approaches. Limnologica-Ecology and Management of Inland Waters, 29(3):249-254

Paerl H W. 2006. Assessing and managing nutrient-enhanced eutrophication in estuarine and coastal waters:Interactive effects of human and climatic perturbations. Ecological Engineering, 26(1):40-54

Pattan J N, Shane P. 1999. Excess aluminum in deep sea sediments of the Central Indian Basin. Marine Geology, 161(2-4):247-255

Saito C, Noriki S, Tsunogai S. 1992. Particulate flux of Al, a component of land origin, in the western North Pacific. Deep-Sea Research Part A. Oceanographic Research Papers, 39(7-8):1315-1327

Schmitz B. 1987. Barium, equatorial high productivity, and the northward wandering of the Indian continent. Paleoceanography, 2(1):63-77

Schropp S J, Lewis F G, Windom H L, et al. 1990. Interpretation of metal concentrations in estuarine sediments of Florida using aluminum as a reference element. Estuaries, 13(3):227-235

Shimmield G B, Mowbray S R, Weedon G P. 1990. A 350 ka history of the Indian Southwest Monsoon-evidence from deep-sea cores, northwest Arabian Sea. Transactions of the Royal Society of Edinburgh:Earth Sciences, 81(4):289-299

Taylor S R, McLennan S M. 1985. The Continental Crust:Its composition and evolution.Oxford:Blackwell Scientific Publications Timothy D A, Calvert S E. 1998. Systematics of variations in excess Al and Al/Ti in sediments from the central equatorial Pacific. Paleoceanograpy, 13(2):127-130

Walsh I, Dymond J, Collier R. 1988. Rates of recycling of biogenic components of settling particles in the ocean derived from sediment trap experiments. Deep-Sea Research Part A. Oceanographic Research Papers, 35(1):43-58

Wang Kai, Feng Shizuo, Shi Xinhui. 2001. A 3-D baroclinic model of summer circulation in the Bohai, Yellow and East China Seas.Oceanologia et Limnologia Sinica (in Chinese), 32(5):551-560

Wang Zhaowei, Ren Jingling, Zhang Guiling, et al. 2015. Behavior of dissolved aluminum in the Huanghe (Yellow River) and its estuary:Impact of human activities and sorption processes. Estuarine, Coastal and Shelf Science, 153:86-95

Wayne Nesbitt H, Markovics G. 1997. Weathering of granodioritic crust, long-term storage of elements in weathering profiles, and petrogenesis of siliciclastic sediments. Geochimica et Cosmochimica Acta, 61(8):1653-1670

Wei Gangjian, Liu Ying, Li Xianhua, et al. 2003a. Climatic impact on Al, K, Sc and Ti in marine sediments:evidence from ODP Site 1144, South China Sea. Geochemical Journal, 37(5):593-602

Wei Gangjian, Liu Ying, Li Xianhua, et al. 2003b. Excess Al in the sediments from South China Sea. Bulletin of Mineralogy, Petrology and Geochemistry (in Chinese), 22(1):23-25

Xu Gang, Liu Jian, Pei Shaofeng, et al. 2014. Distribution and source of heavy metals in the surface sediments from the near-shore area, north Jiangsu Province, China. Marine Pollution Bulletin, 83(1):275-281

Yang Shouye, Li Congxian. 1999. Element composition and tracing in the modern Yangtze River and Yellow River. Progress in Natural Science (in Chinese), 9(10):930-937

Yang Shouye, Jung H S, Li Congxian, et al. 2004. Major element geochemistry of sediments from Chinese and Korean rivers.Geochimica (in Chinese), 33(1):99-105

Zhou Guohua, Sun Binbin, Zeng Daoming, et al. 2014. Vertical distribution of trace elements in the sediment cores from major rivers in east China and its implication on geochemical background and anthropogenic effects. Journal of Geochemical Exploration, 139:53-67

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山东半岛北部滨浅海区表层沉积物铝物源鉴别

doi: 10.1007/s13131-015-0766-9

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Source identification of aluminum in surface sediments of the Yellow Sea off the Shandong Peninsula

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